Évaluation des Radionucléides Terrestres et du Risque Radiologique dans les Matériaux de Construction Indigènes : Une Étude de Cas du District de Liwale, Tanzanie
DOI:
https://doi.org/10.15392/2319-0612.2026.3053Palavras-chave:
Radionuclídeos naturais, Riscos de radiação em interiores, Materiais de construçãoResumo
L’exposition prolongée aux rayonnements ionisants en milieu intérieur constitue un enjeu majeur de santé publique, principalement en raison de la présence de radionucléides naturels dans les matériaux de construction. Cette étude a été entreprise à la suite de la documentation de niveaux élevés de rayonnement gamma dans le district de Liwale. L’objectif est d’évaluer la radioactivité naturelle et les risques radiologiques associés aux matériaux de construction issus de cette région, caractérisée par des Arénosols hypoluviques et des Luvisols profondiques/aréniques dérivés de dépôts de grès néogènes continentaux. Vingt-cinq échantillons de sable, d'argile et de gravier ont été analysés par spectrométrie gamma à l’aide d’un détecteur au germanium de haute pureté (HPGe). Les concentrations d'activité moyennes mesurées pour le 226Ra, le 232Th et le 40K étaient respectivement de 40.8±2.5 Bq kg-1, 114.9±4.1 Bq kg-1 et 311.9±14.5 Bq kg-1. Bien que les niveaux de 40K soient conformes aux normes, les concentrations de 226Ra et de 232Th dépassent les moyennes mondiales de l'UNSCEAR. L'évaluation des indices de risque radiologique indique des valeurs moyennes (Raeq, 229.1±9.6 Bq kg-1; Hex, 0.6; I, 0.8, et Eff, 0.5 mSv an-1) situées en deçà des limites internationales recommandées, suggérant un risque globalement faible. Toutefois, une analyse individuelle révèle que 20 % des échantillons (5 sur 25) excèdent les seuils de sécurité pour Raeq, Hex, et I, tandis que 16 % (4 sur 25) dépassent la limite de dose efficace annuelle (Eff). Ces résultats mettent en évidence des risques lithogéniques potentiels liés à l'utilisation de ces matériaux de construction. En conséquence, cette étude préconise la mise en œuvre rigoureuse de mesures réglementaires de contrôle et de dépistage des matériaux de construction issus de ces formations géologiques spécifiques.
Downloads
Referências
[1] KOVLER, K.; TSAPALOV, A.; BOBKIER, R.; WIEGERS, R.; SCHROEYERS, W.; KOVÁCS, T.; TOTH-BODROGI, E.; EL BOUNAGUI, O.; BABCZUK, A. Indoor radon and NORM in building materials: Critical analysis of the current European regulation and road map for the next decade. J Environ Radioactiv, Berlin, v. 285, n. 107668, p. 1-8, 2025. DOI: https://doi.org/10.1016/j.jenvrad.2025.107668
[2] IMANI, M.; ADELIKHAH, M.; SHHROKHI, A.; AZIMPOUR, G.; YADOLLAHI, A.; KOCSIS, E.; TOTH-BODROGI, E.; KOVACS, T. Natural radioactivity and radiological risks of common building materials used in Semnan Province dwellings Iran. Environ. Sci. Pollut. Res. Int, Berlin, v. 28, p. 41492-41503, 2021. DOI: https://doi.org/10.1007/s11356-021-13469-6
[3] ESTOKOVA, A.; SINGOVSZKA, E.; VERTAL, M. Investigation of building materials’ radioactivity in a historical building—a case study. Materials, Basel, v. 15, n. 19, p. 1-19, 2022. DOI: https://doi.org/10.3390/ma15196876
[4] International Atomic Energy Agency (IAEA). In: IAEA. Regulatory and management approaches for the control of environmental residues containing naturally occurring radioactive material (NORM). Vienna, 2006. p. 1-131. ISBN 92-0-113305-7.
[5] MAS, J. L.; RAMIREZ, J. R. C.; BERMUDEZ, S. H.; FERNANDEZ, C. L. Assessment of natural radioactivity levels and radiation exposure in new building materials in Spain. Radiat Prot Dosimetry, Oxford, v. 194, n. 2-3, p. 178-185, 2021. DOI: https://doi.org/10.1093/rpd/ncab089
[6] SAMREH, M. M. A.; THABAYNEH, K. H.; KHRAIS, F. W. Measurement of activity concentration levels of radionuclides in soil samples collected from Bethlehem Province, West Bank, Palestine. Turkish J Eng Env Sci, Ankara, v. 38, p. 113-125, 2014. DOI: https://doi.org/10.3906/muh-1303-8
[7] MAMMBA, H.P.; BALOBEGWA, V. A.; MUHULO, A. P.; PANTALEO, P. A.; KAWALA, R. A. Assessment of natural radioactivity and radiation hazards of building materials in Kinondoni District, Dar es Salaam. Tanz. J. Sci, Dar es Salaam, v. 47, n. 2, p. 664-673, 2021. DOI: https://doi.org/10.4314/tjs.v47i2.22
[8] IDRIS, M. M.; UBAIDULLAH, A.; SULAYMAN, M. B.; ABDULLAHI, B.; SIDI, M. A. Assessment of gamma background exposure levels in some selected residential houses in FCT Abuja, Nigeria. J. Rad. Nucl. Appl, Budapest, v. 6, n. 3, p. 245-248, 2021. DOI: https://doi.org/10.18576/jrna/060309
[9] WANG, J.; DU, W.; LEI, Y.; CHEN, Y.; WANG, Z.; MAO, K.; TAO, S.; PAN, B. Quantifying the dynamic characteristics of indoor air pollution using real-time sensors: Current status and future implications. Environment International, Rio de Janeiro, v. 175, n. 107934, p. 1-12, 2023. DOI: https://doi.org/10.1016/j.envint.2023.107934
[10] MARTIN, J.G.; KRAAKMAN, N.J.R.; PEREZ, C.; LEBRERO, R.; MUNOZ, R.; A state–of–the-art review on indoor air pollution and strategies for indoor air pollution control. Chemosphere, Amsterdam, v. 262, n. 128376, 2021. DOI: https://doi.org/10.1016/j.chemosphere.2020.128376
[11] FERGUSON, L.; TAILOT, J.; DAVIES, M.; SHRUBSOLE, C.; SYMONDS, P.; DIMITROULOPOULOU, S. Exposure to indoor air pollution across socio-economic groups in high-income countries: A scoping review of the literature and a modelling methodology. Environment International, Rio de Janeiro, v. 143, n. 105748, 2020. DOI: https://doi.org/10.1016/j.envint.2020.105748
[12] United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), In: UNSCEAR, Sources and effects of ionizing radiation, Report of the United Nations Scientific Committee on the Effects of Atomic Radiation to the General Assembly, New York: United Nations Publication, 2000. v. 1. ISBN 92-1-142238-8.
[13] International Atomic Energy Commission (IAEA), Attribution of radiation health effects and inference of radiation risks, Considerations for Application of the IAEA safety Standards, Safety Report Series No. 122. Vienna: IAEA Publishing Section, 2023.p. 25-39. ISBN 978-92-0-134323-9.
[14] MOHAMMED, K.H.; ZYUGHIR, L.S.; JAAFAR, A.A.; ALMAYAHI, B.A. Biological effect of background radiation and their risk of humans. Maghreb. J. Pure & Appl. Sci, Ouja, v. 2, n. 2, p. 71-78, 2016.
[15] RIBEIRO, F.C.A.; LAURIA, D.C.; SILVA, J.I.R.; LIMA, E.S.A.; SABRINHO, N.M.B.A. Baseline and quality reference values for natural radionuclides in soils of Rio de Janeiro State, Brazil. Rev.Bras.Cienc.Solo, Viçosa, v. 42, n. e0170146, p. 1-15, 2018. DOI: https://doi.org/10.1590/18069657rbcs20170146
[16] LEGASU, M. L.; CHAUBEI, A.K. Determination of dose derived from building materials and radiological health related effects from the indoor environment of Dessie city, Wollo, Ethiopia. Heliyon, v. 8, n. 3, p. 1-9, 2022. DOI: https://doi.org/10.1016/j.heliyon.2022.e09066
[17] Directorate-General for Environment (European Commission), Radiological protection principles concerning the natural radioactivity of building materials. Radiation Protection 112, EC, STUK Finland, 1999.
[18] International Commission on Radiological Protection (ICRP), SMITH, H. In: ICRP, 1990 Recommendations of the international commission on radiological protection. New York: Pergamon Press, 1991. ISBN 0 08 041144 4.
[19] KASHKINBAYEV, Y.; KAZHIYAKHMETOVA, B.; ALTAEVA, N.; BAKHTIN, M.; TARLYKOV, P.; SAIFULINA, E.; AUMALIKOVA, M.; IBRAYEVA, D.; BOLATOV, A. Radon exposure and cancer risk: Assessing genetic and protein markers in affected populations. Biology, Basel, v. 15, n. 506, p. 1-20, 2025. DOI: https://doi.org/10.3390/biology14050506
[20] RESTE, J.; RIMERE, N.; ROMANS, A.; MARTINSONE, Z.; MARTINSONE. I.; VANADZINS, I.; PAVLOVSKA, I. Assessment of indoor radon gas concentration in Latvian households. Atmosphere, Basel, v. 15, n. 5, p. 1-12, 2024. DOI: https://doi.org/10.3390/atmos15050611
[21] Tanzania Atomic Energy Commission (TAEC). Internal Technical Report: Radiological Survey of Residential Dwellings in Liwale District. Directorate of Radiation Control Unit, Dodoma, Tanzania (Unpublished). 2023.
[22] DONDEYNE, S.; NGATUNGA, E.L.; COOLS, N.; MUGOGO, S.; DECKERS, J. Landscapes and soils of South Eastern Tanzania: their suitability for cashew. Presented at the 19th conference of the Soil Science Society of East Africa, Moshi, 2001.
[23] THE COUNCIL OF THE EUROPEAN UNION (EU). laying down basic safety standards for protection against the dangers arising from exposure to ionising radiation, and repealing Directives 89/618/Euratom, 90/641/Euratom, 96/29/Euratom, 97/43/Euratom and 2003/122/Euratom. Official Journal of the European Union, Brussels, 2013.
[24] ILORI, A. O.; CHETTY, N.; ADELEYE, B. Assessment of radiological hazard indices due to natural radionuclides in the soil of Irele Local Government Area, Ondo State, Nigeria. Environ. Forensics, London, v. 25, n. 4, p. 173-179, 2023. DOI: https://doi.org/10.1080/15275922.2023.2172096
[25] LOLILA, F.; MAZUNGA, M. S. Measurements of natural radioactivity and evaluation of radiation hazard indices in soils around the Manyoni uranium deposit in Tanzania. J. Radiat. Res. Appl. Sci, Abingdon, v. 16, n. 100524, p. 1-9, 2023. DOI: https://doi.org/10.1016/j.jrras.2023.100524
[26] WANG, Z.; YE, Y. Assessment of Soil radioactivity levels and radiation hazards in Guangyao Village, South China. J. Radioanal. Nucl, Bavaria, v. 329, p. 679-693, 2021. DOI: https://doi.org/10.1007/s10967-021-07818-5
[27] MOSTAFA, A. M. A.; ISSA, S. Natural radioactivity and radiological hazards in some building materials used in new Assiut City, Egypt. Anglisticum, Basel, v. 1, n. 1, p. 321-327, 2013.
[28] RANI, A.; SINGH, S. Natural radioactivity in soil samples from some areas of Himachal Pradesh, India using ɤ-ray spectrometry. Atmos. Environ, Amsterdam, v. 39, p. 6306-6314, 2005. DOI: https://doi.org/10.1016/j.atmosenv.2005.07.050
[29] HASSAN, N. N.; KHOO, K. S. Measurement of natural radioactivity and assessment of radiation hazard indices in soil samples at Pengerang, Kota Tinggi, Johor. AIP Publishing, New York, v. 1584, p. 190-195, 2014. DOI: https://doi.org/10.1063/1.4866130
[30] ISMAIL, A. F.; ABDULLAHI, S.; SAMAT, S.; YASIR, M. S. Radiological dose assessment of natural radioactivity in Malaysian tiles using ResRad-Build computer code. Saints Malaysiana, Selangor, v. 47, n. 5, p. 1017-1023, 2018. DOI: https://doi.org/10.17576/jsm-2018-4705-18
[31] BANZI, F. P.; MSAKI, P. K.; MOHAMMED, N. K. Assessment of natural radioactivity in soil and its contributions to population exposure in the vicinity of Mkuju River Uranium Project in Tanzania. Expert Opin Environ Biol, London, v. 5, n. 4, p. 1-10, 2017. DOI: https://doi.org/10.4172/2325-9655.1000140
[32] Statistician General, National Bureau of Statistics and Office of Chief Government Statistician, Population and Housing Census 2012. Population distribution by administrative areas, Dar es Salaam, 2022.
[33] ASADUZZAMAN, K.; MANNAN, F.; KHANDAKER, M. U.; FAROOK, M. S.; ELKEZZA, A.; AMIN, Y. B. M. Assessment of natural radioactivity levels and potential radiological risks of rommon building materials used in Bangladeshi Dwellings. PLOS ONE, California, v. 10, p. 1-16, 2015. DOI: https://doi.org/10.1371/journal.pone.0140667
[34] JEONG, M.; LEE, K. B.; KIM, K. J.; LEE, M.; HAN, J. Gamma-ray full spectrum analysis for environmental radioactivity by HPGe detector. J aston Space Sci, Texas, v. 31, p. 317-323, 2014. DOI: https://doi.org/10.5140/JASS.2014.31.4.317
[35] AYENI, D. A.; ADEBIYI, F. M. Evaluation of natural radioactivity and radiation hazards of soils around petroleum products marketing company using gamma ray spectrometry. Tanz. J. Sci, Dar es Salaam, v. 48, n. 2, p. 304-312, 2022. DOI: https://doi.org/10.4314/tjs.v48i2.7
[36] JOEL, E. S.; MAXWELL, O.; ADEWOYIN, O. O.; EHI-EROMOSELE, C. O.; EMBONG, Z.; OYAWOYE, F. Assessment of natural radioactivity in various commercial tiles used for building purposes in Nigeria. MethodsX, Sandtone, v. 5, p. 8-19, 2018. DOI: https://doi.org/10.1016/j.mex.2017.12.002
[37] JEAN-CLAUDE, B.O.; ALFRED, A. D. D.; ALAIN, M. G. Assessment of natural radioactivity in gravel samples collected from Abidjan district in Côte d’Ivoire. EJAS, Basel, v. 10, p. 125-134, 2022. DOI: https://doi.org/10.14738/aivp.101.11558
[38] PETOUSSI-HENSS, N.; SATOH, D.; ENDO, A.; ECKERMAN, K. F.; BOLCH, W. E.; HUNT, J.; JANSEN, J. T. M.; KIM, C. H.; LEE, C.; SAITO, K.; SCHLATTL, H.; YEOM, Y. S.; YOO, S. J. International Commission on Radiological Protection (ICRP). In: CLEMENT, C. H, FUJITA, H. Dose Coefficients for external exposure to environmental sources. ICRP Publication 144. Ann. ICRP (49)(2). Ottawa: SAGE, 2020. p. 29-35. ISBN 9781529741254. DOI: https://doi.org/10.1177/0146645320906277
[39] International Atomic Energy Agency (IAEA), In: IAEA. Naturally occurring radioactive materials (NORM VII), Vienna, 2015. ISBN 978-92-0-104014-5.
[40] AKRAM, M.; TURKI, I. E. Radiological assessment of hazard index for clay sample in Iraq. IJONS, Tamil Nadu, v. 9, p. 16417-16424, 2019.
[41] ZIVUKU, M.; KGABI, N. A.; Tshivhase, V. M. Assessment of radioactivity in particulate matter and soil from selected mining towns of Erongo region, Namibia. Scientific African, v. 20, n. e01722, p. 1-10, 2023. DOI: https://doi.org/10.1016/j.sciaf.2023.e01722
[42] RAVISANKAR, R.; CHANDRAMOHAN, J.; CHANDRASEKARAN, A.; JEBAKUMAR, J. P. P.; VIJAYALAKSHMI, I.; VIJAYAGOPAL, P.; VENKATRAMAN, B. Assessments of radioactivity concentration of natural radionuclides and radiological hazard indices in sediment samples from the East coast of Tamilnadu, India with statistical approach. Mar. Pollut. Bull, Qingdao, v. 97, n. 1-2, p. 419-430, 2015. DOI: https://doi.org/10.1016/j.marpolbul.2015.05.058
[43] OSMAN, R.; DAWOOD, Y. H.; MELEGY, A.; EL-BADY, M. S.; SALEH, A.; GAD, A. Distributions and risk assessment of the natural radionuclides in the soil of Shoubra El Kheima, South Nile Delta, Egypt. MDPI Journal, Basel, v. 13, n.1, p. 1-16, 2022. DOI: https://doi.org/10.3390/atmos13010098
[44] CHEN, T.; ZENG, F.; LIN, C.; YEH, Y.; HUANG, W. Assessment of soil radioactivity associated with risk and correlation with soil properties near Maanshan Nuclear Power Plant, Taiwan. Applied Sciences, California, v. 14, n. 20, p. 1-15, 2024. DOI: https://doi.org/10.3390/app14209239
[45] TURHAN, S. Radiological impacts of the usability of clay and kaolin as raw material in manufacturing of structural building materials in Turkey. J. Radiol. Prot, Bristol, v. 29, p. 75-83, 2009. DOI: https://doi.org/10.1088/0952-4746/29/1/005
[46] HARB, S.; EL-KAMEL, A. H.; ZAHRAN, A. M.; ABBADY, A.; AHMED, F. A. Assessment of natural radioactivity in soil and water samples from Aden governorate South of Yemen region. Int. J. Recent Res. Phys. Chem. Sci, Lucknow, v. 1, p. 1-7, 2013.
[47] EL-TAHER, A. Assessment of natural radioactivity levels and radiation hazards for building materials used in Qassim area, Saudi Arabia. Rom. Journ. Phys, Bucharest, v. 57, n. 3-4, p. 726-735, 2012.
[48] OBORAH, K. A.; HASHIM, N. O.; MIGWI, C. M.; ROTICH, C. Assessment of radioactivity concentration for building materials used in Babadogo Estate, Nairobi City County, Kenya. Radiat Prot Dosimetry, Oxford, v. 200, n. 2, p. 201-205, 2023. DOI: https://doi.org/10.1093/rpd/ncad293
[49] KIDANE, Y. B.; DERESSU, T. T.; BELETE, G. D. Evaluation of natural radioactivity level in surface soil from Bambasi district in Benishangul Gumuz region, Ethiopia. J. Anal. Methods CheM, New Jersey, v. 2024, p. 1-14, 2024. DOI: https://doi.org/10.1155/2024/6633673
Downloads
Publicado
Declaração de Disponibilidade de Dados
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Edição
Seção
Licença
Direitos autorais (c) 2026 Huruma Peter Mammba, Machibya A. Anthony

Este trabalho está licenciado sob uma licença Creative Commons Attribution 4.0 International License.
Declaro que o presente artigo é original, não tendo sido submetido à publicação em qualquer outro periódico nacional ou internacional, quer seja em parte ou em sua totalidade. Declaro, ainda, que uma vez publicado na revista Brazilian Journal of Radiation Sciences, editada pela Sociedade Brasileira de Proteção Radiológica, o mesmo jamais será submetido por mim ou por qualquer um dos demais co-autores a qualquer outro periódico. Através deste instrumento, em meu nome e em nome dos demais co-autores, porventura existentes, cedo os direitos autorais do referido artigo à Sociedade Brasileira de Proteção Radiológica, que está autorizada a publicá-lo em meio impresso, digital, ou outro existente, sem retribuição financeira para os autores.
Licença
Os artigos do BJRS são licenciados sob uma Creative Commons Atribuição 4.0 Licença Internacional, que permite o uso, compartilhamento, adaptação, distribuição e reprodução em qualquer meio ou formato, desde que você dê o devido crédito ao (s) autor (es) original (is) e à fonte, forneça um link para a licença Creative Commons, e indique se mudanças foram feitas. As imagens ou outro material de terceiros neste artigo estão incluídos na licença Creative Commons do artigo, a menos que indicado de outra forma em uma linha de crédito para o material. Se o material não estiver incluído no licença Creative Commons do artigo e seu uso pretendido não é permitido por regulamentação legal ou excede o uso permitido, você precisará obter permissão diretamente do detentor dos direitos autorais. Para visualizar uma cópia desta licença, visite http://creativecommons.org/licenses/by/4.0/






















